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Numerical and experimental study of radiation induced conductivity change of carbon nanotube filled polymers
Liu, Fangjun1; Sun, Yonghai2,3; Sun, Weijie1; Sun, Zhendong4; Yeow, John T. W.2,3
2017-06-23
发表期刊NANOTECHNOLOGY
ISSN0957-4484
卷号28期号:25页码:10
摘要Measuring the conductivity changes of sensing materials to detect a wide range of radiation energy and dosage is one of the major sensing mechanisms of radiation sensors. Carbon nanotube (CNT) filled composites are suitable for sensing radiation because of the extraordinary electrical properties of CNTs and the CNT-network formed inside the polymer matrix. Although the use of CNT-based nanocomposites as potential radiation sensing materials has been widely studied, there is still a lack of theoretical models to analyze the relationship between electrical conductivity and radiation dosages. In this article, we propose a 3D model to describe the electrical conductivity of CNT-based nanocomposites when being irradiated by ionizing radiation. The Monte Carlo method has been employed to calculate radiation intensity, CNT concentration and alignment's influence on the electrical conductivity. Our simulation shows a better agreement when CNT loading is between the percolation threshold and 3% volume fraction. Radiation experiments have been performed to verify the reliability of our model to illustrate a power function relationship between the electrical conductivity of a CNT-filled polymer and radiation intensity. In addition, the predicted alignment to obtain the best sensitivity for radiation sensing has been discussed to help with CNT-network building in the fabrication process.
关键词carbon nanotube electrical conductivity radiation sensor 3D model alignment
DOI10.1088/1361-6528/aa701e
语种英语
资助项目Chinese Scholarship Council ; Natural Sciences and Engineering Research Council of Canada (NSERC) ; Canada Research Chairs Program
WOS研究方向Science & Technology - Other Topics ; Materials Science ; Physics
WOS类目Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied
WOS记录号WOS:000402893900001
出版者IOP PUBLISHING LTD
引用统计
文献类型期刊论文
条目标识符http://ir.amss.ac.cn/handle/2S8OKBNM/25663
专题系统科学研究所
通讯作者Yeow, John T. W.
作者单位1.South China Univ Technol, Sch Automat Sci & Engn, Guangzhou 510641, Guangdong, Peoples R China
2.Univ Waterloo, Dept Syst Design Engn, Waterloo, ON N2L 3G1, Canada
3.Univ Waterloo, Waterloo Inst Nanotechnol, Waterloo, ON N2L 3G1, Canada
4.Chinese Acad Sci, Acad Math & Syst Sci, Key Lab Syst & Control, Beijing 100190, Peoples R China
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GB/T 7714
Liu, Fangjun,Sun, Yonghai,Sun, Weijie,et al. Numerical and experimental study of radiation induced conductivity change of carbon nanotube filled polymers[J]. NANOTECHNOLOGY,2017,28(25):10.
APA Liu, Fangjun,Sun, Yonghai,Sun, Weijie,Sun, Zhendong,&Yeow, John T. W..(2017).Numerical and experimental study of radiation induced conductivity change of carbon nanotube filled polymers.NANOTECHNOLOGY,28(25),10.
MLA Liu, Fangjun,et al."Numerical and experimental study of radiation induced conductivity change of carbon nanotube filled polymers".NANOTECHNOLOGY 28.25(2017):10.
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